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4GB is generally a must have for Vista 64, especially if its gonna be used for gaming or anything with lots of Ram usage, for 32 bit you could get away with 2GB (but then you'd only be able to use 3GB anyway).
The Kingston Ram won't be of much benefit unless you intend on OCing past 400MHz FSB as well (and even then is probably overkill, PC8500 (1066Mhz) would be plenty.
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