TwinMOS memory modules are rated at 2.8v, much more than the 2.6v that you're most likely putting thru the memory, that's probably the reason for you not being able to hit 200fsb. When I had TwinMOS PC3200, it was rated at 200FSB 2.5-3-3-7, altho it was CH-5 so it would do 200FSB at 2-3-2-6 with 2.9v vDIMM, that's well within the +-5% that the manufacturers allow for with warranty so you'll have no problems there.
You need to lower the multiplier and then increase the front side bus, set the memory divider to 3/3 or 5/5 they're the fastest dividers on nForce2 from my experiences in benchmarking and tweaking. You also need to keep the memory bus in sync with the front side bus (using either the 3/3 or 5/5 dividers) for the best performance on AMD based systems. The nForce2 platform's bandwidth already saturates the Athlon XP's bus as it's already double the speed, so increasing the memory bus past the front side bus (CPU external clock) will actually cause a performance drop. You will get great memory bandwidth, but with an already saturated front side bus, you'll get no extra performance from the system.
Set the Multiplier to 8.0x front side bus to 166 and then see what happens there. TwinMOS is weird stuff
tbh, took me a while to get the best out of it. I was having trouble getting past 192fsb at first, then all of a sudden something clicked, can't remember what it was but it solved my problems of getting above 192fsb, all of a sudden I could get up to 218fsb on it's rated 2.5-3-3-7 timings.
Hope this helps you a bit, good luck with it and don't be afraid to ask more questions. I'll try my best to help.
bigZ