With the NF7 boards with the newer Bios there was an option when the mobo detected an X2500 to either run it at 2500 speeds or 3200 speeds ie 11x166 or 11x200 you could just select what you wanted.Or you can use user defined
I would look at putting the vcore around 1.75 some even have it at 1.85 but I wouldn't go much higher.
Set the FSB/dram ratio to 6/6
One thing you haven't mentioned is what PSU you are using, with that card you have a big draw on the power and putting up the FSB may just be the straw that breaks the camels back